10.6084/m9.figshare.11439987.v1
Shuo Zhang
Shuo
Zhang
Jiyan Liang
Jiyan
Liang
Xinyang Yu
Xinyang
Yu
Tao Xu
Tao
Xu
Xinjun Shen
Xinjun
Shen
Post-plasma-catalytic degradation of toluene using atmosphere double dielectric barrier discharge combined MnO<i><sub>x</sub></i>-based catalysts
Taylor & Francis Group
2019
Post-plasma catalytic system
toluene
Ce1Mn1/Al2O3 catalyst
double dielectric barrier discharge
2019-12-23 12:23:48
Journal contribution
https://tandf.figshare.com/articles/journal_contribution/Post-plasma-catalytic_degradation_of_toluene_using_atmosphere_double_dielectric_barrier_discharge_combined_MnO_i_sub_x_sub_i_-based_catalysts/11439987
<p>Post-plasma catalytic system with Mn-based has shown potential performance in terms of air pollution degradation, in which Ce was induced into MnOx/Al<sub>2</sub>O<sub>3</sub> mixed with 1:1 weight ratio by the impregnation method to increase the capacity of toluene degradation. The catalytic ability of prepared catalysts was analyzed by characterizations of XRD, SEM, XPS, and BET. The effects of the SIE and initial concentration on toluene and CO<sub>2</sub> production were discussed in this work. The results showed that the toluene removal efficiency and CO<sub>2</sub> selectivity increased with the promotion of SIE. With the addition of 15% Ce1Mn1/A<sub>2</sub>O<sub>3</sub>, the PPC system displayed the potential performance in the enhancement of toluene conversion and CO<sub>2</sub> generation, and suppression of ozone and NO<sub>2</sub> compared with plasma alone. At the SIE level of 504 J/L, the system showed better performance in terms of toluene removal efficiency (90.1%), CO<sub>2</sub> selectivity (67.3%), O<sub>3</sub> suppression (79.3%), and NO<sub>2</sub> prohibition (61.8%). Also, the organic by-products generated by the PPC system were discussed.</p>